So I called our water supply quality control place. They said Pennsburg is a large area, therefore, GH ranges from 142 mg/L to 200mg/L.
This helps. With the GH this low, I would not maintain livebearers, there simply is not sufficient dissolved mineral (primarily calcium and magnesium) in the water. If your GH is at the upper end of the given range, it should bee OK, but if it is below that, certainly not. So I would not consider more livebearers. The other fish are fine. The pH is OK, and if it lowers which it might, that's OK too (for the other fish, not livebearers).
I've watched the videos, and read your posts again, and I would suggest first that the softish water has weakened the platies which makes them more susceptible to problems. I would also suggest that the chasing by the red tail shark is undoubtedly part of the problem; I realize you are attempting to re-home it, and that cannot be done fast enough. This species once it takes a dislike to any other fish is relentless until that fish/those fish are dead.
I do not generally get involved in disease issues as I have so little experience (fortunately) and thus little researched knowledge in this area. But there are always some general observations one can make, as Colin did about water changes, etc. And here I would say the platy is not going to recover no matter what you do, so euthanization would be kinder in the long-term. The male is pestering her, which is more stress, on top of the shark. When fish develop the swimming this platy is doing, I have never heard of recovery because, according to a marine biologist I know, the internal damage caused by whatever is permanent. Treating the tank for this or that which is highly unlikely to help this fish is only causing more trouble because any additive to the water gets inside all the fish, and unless this is absolutely essential it should not occur. Water changes, fine, with a good conditioner, nothing else.